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Investigating photoresponsivity of graphene-silver hybrid nanomaterials in the ultraviolet

2020

Article

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There have been several reports of plasmonically enhanced graphene photodetectors in the visible and the near infrared regime but rarely in the ultraviolet. In a previous work, we have reported that a graphene-silver hybrid structure shows a high photoresponsivity of 13 A/W at 270 nm. Here, we consider the likely mechanisms that underlie this strong photoresponse. We investigate the role of the plasmonic layer and examine the response using silver and gold nanoparticles of similar dimensions and spatial arrangement. The effect on local doping, strain, and absorption properties of the hybrid is also probed by photocurrent measurements and Raman and UV-visible spectroscopy. We find that the local doping from the silver nanoparticles is stronger than that from gold and correlates with a measured photosensitivity that is larger in devices with a higher contact area between the plasmonic nanomaterials and the graphene layer.

Author(s): Deshpande, P. and Suri, P. and Jeong, H.-H. and Fischer, P. and Ghosh, A. and Ghosh, G.
Journal: J. Chem. Phys.
Volume: 152
Pages: 044709
Year: 2020
Month: January
Day: 27

Department(s): Micro, Nano, and Molecular Systems
Bibtex Type: Article (article)

DOI: https://doi.org/10.1063/1.5138722
URL: https://doi.org/10.1063/1.5138722

BibTex

@article{Ghosh2020,
  title = {Investigating photoresponsivity of graphene-silver hybrid nanomaterials in the ultraviolet},
  author = {Deshpande, P. and Suri, P. and Jeong, H.-H. and Fischer, P. and Ghosh, A. and Ghosh, G.},
  journal = {J. Chem. Phys.},
  volume = {152},
  pages = {044709},
  month = jan,
  year = {2020},
  url = {https://doi.org/10.1063/1.5138722},
  month_numeric = {1}
}